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Creators/Authors contains: "Underhill, Patrick T."

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  1. Complex fluid interfaces are commonplace in natural and engineered systems and a major topic in the fields of rheology and soft matter physics, providing boundary conditions for a system’s hydrodynamics. The relationship between structure and function dictates how constituents within complex fluids govern flow behavior via constituents changing conformation in response to the local microenvironment to minimize free energy. Both hydrodynamics, such as shear flow, and the presence of air–liquid interfaces are principal aspects of a complex fluid’s environment. The study of fluid interfaces coupled to bulk flows can be uniquely advanced through experimentation in microgravity, where surface tension containment can be achieved at relatively large length scales. This computational investigation assesses flow in the ring-sheared drop (RSD), a containerless biochemical reactor operating aboard the International Space Station for the study of complex fluids and soft matter physics. Specifically, the hydrodynamic effects of a generalized Boussinesq–Scriven interface with a shear-thinning surface shear viscosity are examined in flow regimes where the air–liquid interface remains coupled to the Newtonian bulk fluid. The results verify this interfacial model’s ability to affect system-wide hydrodynamics under specific parameter regimes, enabling future model validation with high-precision rheological measurements. 
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    Free, publicly-accessible full text available February 26, 2026
  2. We review the literature on swimming in complex fluids. A classification is proposed by comparing the length- and timescales of a swimmer with those of nearby obstacles, interpreted broadly, extending from rigid or soft confining boundaries to molecules that confer the bulk fluid with complex stresses. A third dimension in the classification is the concentration of swimmers, which incorporates fluids whose complexity arises purely by the collective motion of swimming organisms. For each of the eight system types that we identify, we provide a background and describe modern research findings. Although some types have seen a great deal of attention for decades, others remain uncharted waters still open and awaiting exploration. 
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  3. In this work, we analyzed an isotropic colloidal model incorporating both short-range sticky attractions and long-range electrostatic repulsions. We computed the zero-shear viscosity and second virial coefficient for a dilute colloidal suspension (i.e., pair interactions only) as a function of the strength of attractions and repulsions. We also developed an analytical approximation that allows us to better understand the coupling of the two types of interactions. The attractions and repulsions contribute to the zero-shear viscosity and second virial coefficient in different ways, leading to cases with the same second virial coefficient but different zero-shear viscosity. The analytical approximation shows that the mechanism of the coupling of interactions is that long-range repulsions can weaken the influence of short-range attractions. This effect alters how repulsions change the zero-shear viscosity. Acting independently, both attractions and repulsions increase the viscosity coefficient of the system. However, when both types of interactions are considered together, repulsions can screen the effect of attractive interactions, thereby reducing the viscosity. 
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